Determination of quinolizidine alkaloids in traditional Chinese herbal drugs by nonaqueous capillary electrophoresis

J Chromatogr A. 1999 Oct 1;857(1-2):303-11. doi: 10.1016/s0021-9673(99)00758-x.

Abstract

A rapid method for the determination of quinolizidine alkaloids by nonaqueous capillary electrophoresis was developed. A total of 10 alkaloids (matrine, sophocarpine, oxymatrine, oxysophocarpine, sophoridine, cytisine, sophoramine, aloperine, lehmannine and dauricine) could be easily separated within 18 min. A running buffer composed of 50 mM ammonium acetate, 10% tetrahydrofuran and 0.5% acetic acid in methanol was found to be the most suitable for this separation. Five of these alkaloids were selected for further studies. The linear calibration ranges were 2.51-50.1 microg/ml for sophoridine and sophocarpine, 2.71-54.2 microg/ml for matrine, 3.30-65.9 microg/ml for oxymatrine, and 3.10-62.0 microg/ml for oxysophocarpine. The recovery of the five alkaloids was 98.0-101.3% with relative standard deviations from 1.03 to 2.68% (n=5). The limits of detection for all 10 alkaloids were over the range 0.93-2.31 microg/ml. The method was successfully applied to the phytochemical analysis of alkaloid extracts from three commonly used traditional Chinese herbal drugs: Sophora flavescens Ait. (Kushen), S. alopecuroides L. (Kudouzi or Kugancao) and S. tonkinensis Gapnep (Shandougen).

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alkaloids / analysis*
  • Calibration
  • Drugs, Chinese Herbal / chemistry*
  • Electrophoresis, Capillary / methods*
  • Medicine, Chinese Traditional*
  • Quinolizines / chemistry
  • Reference Standards
  • Reproducibility of Results

Substances

  • Alkaloids
  • Drugs, Chinese Herbal
  • Quinolizines