Metabolism of the influenza neuraminidase inhibitor prodrug oseltamivir in the rat

Drug Metab Dispos. 2000 Jul;28(7):737-41.

Abstract

The metabolism of [2-acetyl-(14)C]oseltamivir (GS4104, Ro 64-0796), the prodrug of the novel influenza neuraminidase inhibitor GS4071 (Ro 64-0802), was examined in rats after oral dosing. Intact oseltamivir was observed only in lung and urine, accounting for 37 and 15% of the total radioactivity in these samples, respectively. GS4071 was the major metabolite in plasma, tissues, and urine, and accounted for 32 to 56% of the radioactivity present in these samples. The second most abundant peak in these samples (13-24% of radioactivity) was a novel metabolite (M3). This metabolite was purified from urine of rats dosed orally with oseltamivir and was identified by liquid chromatography-mass spectrometry and NMR as the (R)-omega-carboxylic acid metabolite of oseltamivir. The omega-carboxylic acid metabolite of oseltamivir could not be produced in vitro. However, omega-hydroxylated products of oseltamivir were produced by rat liver microsomes. Both the (R)- and (S)-omega-hydroxylated products were observed, but formation of the (R)-isomer predominated. These data indicated that in the rat, oseltamivir was primarily metabolized to the active influenza neuraminidase inhibitor GS4071 and, to a lesser extent, to an (R)-omega-carboxylic acid metabolite.

MeSH terms

  • Acetamides / pharmacokinetics*
  • Animals
  • Enzyme Inhibitors / pharmacokinetics*
  • Male
  • Microsomes, Liver / metabolism
  • Neuraminidase / antagonists & inhibitors*
  • Oseltamivir
  • Prodrugs / pharmacokinetics*
  • Rats
  • Rats, Sprague-Dawley
  • Reference Standards
  • Tissue Distribution

Substances

  • Acetamides
  • Enzyme Inhibitors
  • Prodrugs
  • Oseltamivir
  • Neuraminidase