Abstract
Compounds containing a 1,2,3-triazole-substituted benzenesulfonamide were prepared and found to be potent and selective human beta3-adrenergic receptor agonists. The most interesting compound, trifluoromethylbenzyl analogue 12e (beta3 EC50 = 3.1 nM with >1500-fold selectivity over binding to both beta1- and beta2 receptors), stimulates lipolysis in the rhesus monkey (ED50 = 0.36 mg/kg) and is 25% orally bioavailable in the dog.
MeSH terms
-
Administration, Oral
-
Adrenergic beta-3 Receptor Agonists*
-
Animals
-
Benzenesulfonamides
-
Biological Availability
-
CHO Cells
-
Cricetinae
-
Cyclic AMP / metabolism
-
Dogs
-
Dose-Response Relationship, Drug
-
Humans
-
Infusions, Parenteral
-
Isoproterenol / pharmacology
-
Lipolysis / drug effects
-
Macaca mulatta
-
Protein Binding
-
Receptors, Adrenergic, beta-3 / metabolism
-
Structure-Activity Relationship
-
Sulfonamides / chemical synthesis
-
Sulfonamides / metabolism
-
Sulfonamides / pharmacokinetics
-
Tachycardia / chemically induced
-
Triazoles / chemical synthesis
-
Triazoles / metabolism
-
Triazoles / pharmacokinetics
Substances
-
Adrenergic beta-3 Receptor Agonists
-
Receptors, Adrenergic, beta-3
-
Sulfonamides
-
Triazoles
-
Cyclic AMP
-
Isoproterenol