Identification of a lipopolysaccharide alpha-2,3-sialyltransferase from Haemophilus influenzae

Mol Microbiol. 2001 Jan;39(2):341-50. doi: 10.1046/j.1365-2958.2001.02204.x.

Abstract

We have identified a gene for the addition of N-acetylneuraminic acid (Neu5Ac) in an alpha-2,3-linkage to a lactosyl acceptor moiety of the lipopolysaccharide (LPS) of the human pathogen Haemophilus influenzae. The gene is one that was identified previously as a phase-variable gene known as lic3A. Extracts of H. influenzae, as well as recombinant Escherichia coli strains producing Lic3A, demonstrate sialyltransferase activity in assays using synthetic fluorescent acceptors with a terminal galactosyl, lactosyl or N-acetyl-lactosaminyl moiety. In the RM118 strain of H. influenzae, Lic3A activity is modulated by the action of another phase-variable glycosyltransferase, LgtC, which competes for the same lactosyl acceptor moiety. Structural analysis of LPS from a RM118:lgtC mutant and the non-typeable strain 486 using mass spectrometry and nuclear magnetic resonance (NMR) spectroscopy confirmed that the major sialylated species has a sialyl-alpha-(2-3)-lactosyl extension off the distal heptose. This sialylated glycoform was absent in strains containing a lic3A gene disruption. Low amounts of sialylated higher molecular mass glycoforms were present in RM118:lgtC lic3A, indicating the presence of a second sialyltransferase. Lic3A mutants of H. influenzae strains show reduced resistance to the killing effects of normal human serum. Lic3A, encoding an alpha-2,3-sialyltransferase activity, is the first reported phase-variable sialyltransferase gene.

MeSH terms

  • Blood Bactericidal Activity
  • Carbohydrate Sequence
  • Electrophoresis, Capillary
  • Haemophilus influenzae / enzymology*
  • Haemophilus influenzae / genetics
  • Haemophilus influenzae / growth & development
  • Humans
  • Lipopolysaccharides / chemistry*
  • Lipopolysaccharides / metabolism*
  • Mass Spectrometry / methods
  • Molecular Sequence Data
  • Mutation
  • Sialyltransferases / genetics*
  • Sialyltransferases / metabolism*

Substances

  • Lipopolysaccharides
  • Sialyltransferases