Identification of alpha-tocopherol oxidation products in triolein at elevated temperatures

J Agric Food Chem. 2001 Mar;49(3):1508-11. doi: 10.1021/jf001142f.

Abstract

The effect of high-temperature treatment on the stability of alpha-tocopherol (1) in triolein was assessed under a reduced-pressure atmosphere (4-40 mbar) simulating the deodorization step of the refining of vegetable oils. A marked degradation of 1 was observed, which increased with increasing temperature (180-260 degrees C) and heating time (20-80 min). The degradation of 1 in triolein at 240 degrees C was inhibited by the addition of the synthetic antioxidant TBHQ or when heating was performed under nitrogen atmosphere, indicating oxidative degradation. The oxidation products were isolated and identified as alpha-tocopherolquinone (2), 4a,5-epoxy-alpha-tocopherolquinone (3), and 7,8-epoxy-alpha-tocopherolquinone (4).

MeSH terms

  • Antioxidants
  • Food Handling / methods
  • Hot Temperature
  • Hydroquinones
  • Oxidation-Reduction
  • Plant Oils*
  • Thermodynamics
  • Triolein / chemistry*
  • Vitamin E / chemistry*

Substances

  • Antioxidants
  • Hydroquinones
  • Plant Oils
  • Triolein
  • Vitamin E
  • 2-tert-butylhydroquinone