Heterologous expression and properties of the gamma-subunit of the Fe-only hydrogenase from Thermotoga maritima

Biochim Biophys Acta. 2001 Jun 1;1505(2-3):209-19. doi: 10.1016/s0005-2728(01)00166-9.

Abstract

Thermotoga maritima is a hyperthermophilic bacterium that contains a complex, heterotrimeric (alpha(beta)gamma) Fe-only hydrogenase. Sequence analysis indicates that the gene encoding the smallest subunit (gamma), hydC, contains a predicted iron-sulfur cluster binding motif. However, characterization of the native gamma-subunit has been hampered by interference from and the inability to separate intact gamma-subunit from the other two subunits (alpha and beta). To investigate the function and properties of the isolated gamma-subunit, the gene encoding HydG was expressed in Escherichia coli. Two forms of the recombinant protein were obtained with molecular masses of 10 and 18 kDa, respectively. Both contained a single [2Fe-2S] cluster based on metal analysis, EPR and UV-visible spectroscopy. NH2-terminal sequencing revealed that the 10 kDa protein is a truncated form of the intact gamma-subunit and lacks the first 65 amino acid residues. The midpoint potential of the 18 kDa form was -356 mV at pH 7.0 and 25 degrees C, as measured by direct electrochemistry, and was pH dependent with a pK(ox) of 7.5 and a pK(red) of 7.7. The oxidized, recombinant gamma-subunit was stable at 80 degrees C under anaerobic conditions with a half-life greater than 24 h, as judged by the UV-visible spectrum of the [2Fe-2S] cluster. In the presence of air the protein was less stable and denatured with a half-life of approx. 2.5 h. The recombinant gamma-subunit was electron transfer competent and was efficiently reduced by pyruvate ferredoxin oxidoreductase from Pyrococcus furiosus, with a Km of 5microM and a Vmax of 9 U/mg. In contrast, native T. maritima hydrogenase holoenzyme and its separated alpha-subunit were much less effective electron donors for the gamma-subunit, with a V(max) of 0.01 U/mg and 0.1 U/mg, respectively.

Publication types

  • Comparative Study
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Amino Acid Sequence
  • Bacterial Proteins / chemistry
  • Bacterial Proteins / genetics*
  • Base Sequence
  • Electron Spin Resonance Spectroscopy
  • Electron Transport
  • Gene Expression Regulation, Enzymologic
  • Hydrogenase / genetics*
  • Hydrogenase / isolation & purification
  • Hydrogenase / metabolism
  • Iron-Sulfur Proteins / genetics*
  • Iron-Sulfur Proteins / isolation & purification
  • Iron-Sulfur Proteins / metabolism
  • Membrane Potentials
  • Molecular Sequence Data
  • Sequence Alignment
  • Thermotoga maritima / enzymology
  • Thermotoga maritima / genetics*

Substances

  • Bacterial Proteins
  • Iron-Sulfur Proteins
  • iron hydrogenase
  • Hydrogenase