Agonist-induced conformational changes in the G-protein-coupling domain of the beta 2 adrenergic receptor

Proc Natl Acad Sci U S A. 2001 May 22;98(11):5997-6002. doi: 10.1073/pnas.101126198. Epub 2001 May 15.

Abstract

The majority of extracellular physiologic signaling molecules act by stimulating GTP-binding protein (G-protein)-coupled receptors (GPCRs). To monitor directly the formation of the active state of a prototypical GPCR, we devised a method to site specifically attach fluorescein to an endogenous cysteine (Cys-265) at the cytoplasmic end of transmembrane 6 (TM6) of the beta(2) adrenergic receptor (beta(2)AR), adjacent to the G-protein-coupling domain. We demonstrate that this tag reports agonist-induced conformational changes in the receptor, with agonists causing a decline in the fluorescence intensity of fluorescein-beta(2)AR that is proportional to the biological efficacy of the agonist. We also find that agonists alter the interaction between the fluorescein at Cys-265 and fluorescence-quenching reagents localized to different molecular environments of the receptor. These observations are consistent with a rotation and/or tilting of TM6 on agonist activation. Our studies, when compared with studies of activation in rhodopsin, indicate a general mechanism for GPCR activation; however, a notable difference is the relatively slow kinetics of the conformational changes in the beta(2)AR, which may reflect the different energetics of activation by diffusible ligands.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Adrenergic beta-Agonists / chemistry*
  • Albuterol / chemistry
  • Binding Sites
  • Cysteine
  • Detergents / chemistry
  • Dobutamine / chemistry
  • Epinephrine / chemistry
  • Fluoresceins
  • Fluorescence
  • Fluorescent Dyes
  • GTP-Binding Proteins / metabolism*
  • Glucosides / chemistry
  • Humans
  • Isoproterenol / chemistry
  • Kinetics
  • Lysine
  • Micelles
  • Mutagenesis, Site-Directed
  • Protein Conformation*
  • Receptors, Adrenergic, beta-2 / chemistry*
  • Receptors, Adrenergic, beta-2 / genetics
  • Stearic Acids / chemistry

Substances

  • Adrenergic beta-Agonists
  • Detergents
  • Fluoresceins
  • Fluorescent Dyes
  • Glucosides
  • Micelles
  • Receptors, Adrenergic, beta-2
  • Stearic Acids
  • Dobutamine
  • stearic acid
  • dodecyl maltoside
  • fluorescein 5-maleimide
  • GTP-Binding Proteins
  • Lysine
  • Cysteine
  • Isoproterenol
  • Albuterol
  • Epinephrine