Is the effect of interleukin-1 on glutathione oxidation in cultured human fibroblasts involved in nuclear factor-kappaB activation?

Antioxid Redox Signal. 2001 Apr;3(2):329-40. doi: 10.1089/152308601300185269.

Abstract

Our understanding of the interleukin-1 (IL-1) signaling molecular mechanisms has recently made considerable progress, with the discovery of the IL-1 receptor-associated kinase and the downstream enzymatic cascade that leads to the activation of nuclear factor-kappaB (NF-kappaB). IL-1 signaling and especially NF-kappaB activation are thought to be redox-sensitive, even though the precise nature and the molecular targets of the oxidants/antioxidants involved remain largely unknown. Here, we investigated the possible role of cellular oxidized/reduced glutathione (GSSG/GSH) balance in IL-1 signaling. We describe a quantitative method based on capillary electrophoresis designed to assay both intracellular GSH and GSSG in adhering fibroblasts. This method allows the GSSG/GSH balance to be followed during IL-1 stimulation. Our data show that IL-1 induces rapid and transient oxidation of intracellular glutathione in human fibroblasts. Using various antioxidants, including pyrrolidine dithiocarbamate and curcumin, we were unable to show a direct relationship between this IL-1-induced glutathione oxidation and NF-kappaB activation. Of the five antioxidants tested, only curcumin was able to inhibit IkappaBalpha degradation upstream and, hence, NF-kappaB DNA-binding activity and NF-kappaB-dependent expression of IL-6 downstream.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antioxidants / pharmacology
  • Binding Sites
  • Blotting, Western
  • Cells, Cultured
  • Curcumin / pharmacology
  • Enzyme Inhibitors / pharmacology
  • Ethylmaleimide / pharmacology
  • Fibroblasts / drug effects*
  • Fibroblasts / metabolism
  • Glutathione / metabolism*
  • Humans
  • Hydrogen Peroxide / pharmacology
  • I-kappa B Proteins / metabolism
  • Interleukin-1 / pharmacology*
  • NF-kappa B / metabolism*
  • Pyrrolidines / pharmacology
  • Reactive Oxygen Species / metabolism
  • Signal Transduction
  • Thiocarbamates / pharmacology

Substances

  • Antioxidants
  • Enzyme Inhibitors
  • I-kappa B Proteins
  • Interleukin-1
  • NF-kappa B
  • Pyrrolidines
  • Reactive Oxygen Species
  • Thiocarbamates
  • pyrrolidine dithiocarbamic acid
  • Hydrogen Peroxide
  • Glutathione
  • Curcumin
  • Ethylmaleimide