N-(2-hydroxypropyl)methacrylamide copolymer-6-(3-aminopropyl)-ellipticine conjugates. Synthesis, in vitro, and preliminary in vivo evaluation

Bioconjug Chem. 2001 Sep-Oct;12(5):711-8. doi: 10.1021/bc0001544.

Abstract

Ellipticine derivatives have potential as anticancer drugs. Their clinical use has been limited, however, by poor solubility and host toxicity. As N-(2-hydroxypropyl)methacrylamide (HPMA) copolymer-anticancer conjugates are showing promise in early clinical trials, a series of novel HPMA copolymer conjugates have been prepared containing the 6-(3-aminopropyl)-ellipticine derivative (APE, NSC176328). Drug was linked to the polymer via GFLG or GG peptide side chains. To optimize biological behavior, HPMA copolymer-GFLG-APE conjugates with different drug loading (total APE: 2.3-7% w/w; free APE: <0.1% w/w) were synthesized. Conjugation of APE to HPMA copolymers considerably increased its aqueous solubility (>10-fold). HPMA copolymer-GG-APE did not liberate drug in the presence of isolated lysosomal enzymes (tritosomes), but HPMA copolymer-GFLG-APE released APE to a maximum of 60% after 5 h. The rate of drug release was influenced by drug loading; lower loading led to greater release. Whereas free APE (35 microg/mL) caused significant hemolysis (50% after 1 h), HPMA copolymer-APE conjugates were not hemolytic up to 300 microg/mL (APE-equiv). As would be expected from its cellular pharmacokinetics, HPMA copolymer-GFLG-APE was >75 times less cytotoxic than free drug (IC(50) approximately 0.4 microg/mL) against B16F10 melanoma in vitro. However, in vivo when tested in mice bearing s.c. B16F10 melanoma, HPMA copolymer-GFLG-APE (1-10 mg/kg single dose, APE-equiv) given i.p. was somewhat more active (highest T/C value of 143%) than free APE (1 mg/kg) (T/C =127%). HPMA copolymer-APE conjugates warrant further evaluation as potential anticancer agents.

Publication types

  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Acrylamides / administration & dosage
  • Acrylamides / chemical synthesis
  • Acrylamides / pharmacokinetics*
  • Animals
  • Antineoplastic Agents, Phytogenic / administration & dosage
  • Antineoplastic Agents, Phytogenic / chemical synthesis
  • Antineoplastic Agents, Phytogenic / pharmacokinetics*
  • Cell Division / drug effects
  • Drug Carriers / administration & dosage
  • Drug Carriers / chemical synthesis
  • Drug Carriers / pharmacokinetics
  • Drug Evaluation, Preclinical
  • Ellipticines / administration & dosage
  • Ellipticines / chemical synthesis
  • Ellipticines / pharmacokinetics*
  • Hemolysis / drug effects
  • Male
  • Methacrylates / administration & dosage
  • Methacrylates / chemical synthesis
  • Methacrylates / pharmacokinetics
  • Mice
  • Mice, Inbred C57BL
  • Neoplasms, Experimental / drug therapy
  • Polymers / administration & dosage
  • Polymers / chemical synthesis
  • Polymers / pharmacokinetics*
  • Solubility
  • Therapeutic Equivalency
  • Tumor Cells, Cultured / drug effects
  • Tumor Cells, Cultured / transplantation

Substances

  • Acrylamides
  • Antineoplastic Agents, Phytogenic
  • Drug Carriers
  • Ellipticines
  • Methacrylates
  • Polymers
  • methacrylamide
  • hydroxypropyl methacrylate