Tetraphenylbenziporphyrin--a ligand for organometallic chemistry

Chemistry. 2001 Dec 3;7(23):5113-7. doi: 10.1002/1521-3765(20011203)7:23<5113::aid-chem5113>3.0.co;2-v.

Abstract

6,11,16,21-Tetraphenylbenziporphyrin (TPBPH)H, an analogue of tetraphenylporphyrin with one of the pyrrole groups replaced by a benzene ring, is formed in good yield in the condensation of the appropriate precursor with pyrrole and benzaldehyde. (TPBPH)H gives organometallic complexes with palladium(II) and platinum(II), [(TPBP)PdII] and [(TPBP)PtII], in which the metal ion is bound in the macrocyclic cavity by three pyrrolic nitrogen atoms and a carbon atom of the benzene ring. In the reaction with silver(I) acetate benziporphyrin does not yield a stable complex but undergoes selective acetoxylation at the internal carbon atom. (TPBPH)H is reversibly reduced to 6-benziphlorin and reacts with a water or methanol molecule to give 6-hydroxy- or 6-methoxy-6-benziphlorin, respectively.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Benzaldehydes / chemistry
  • Crystallography, X-Ray
  • Ligands
  • Magnetic Resonance Spectroscopy
  • Molecular Structure
  • Organometallic Compounds / chemical synthesis
  • Organometallic Compounds / chemistry
  • Palladium / chemistry
  • Platinum / chemistry
  • Porphyrins / chemical synthesis*
  • Porphyrins / chemistry

Substances

  • Benzaldehydes
  • Ligands
  • Organometallic Compounds
  • Porphyrins
  • tetraphenylporphyrin
  • Platinum
  • Palladium
  • benzaldehyde