Determination of purine and pyrimidine bases in DNA by micellar electrokinetic capillary chromatography with electrochemical detection

J Chromatogr A. 2002 Apr 19;954(1-2):267-76. doi: 10.1016/s0021-9673(02)00161-9.

Abstract

A method based on micellar electrokinetic capillary chromatography with electrochemical detection was developed for the determination of cytosine, 5-methylcytosine (5-MC), thymine, adenine, and guanine in the hydrolysates of DNA. The working electrode was fabricated in a novel self-positioning carbon disc electrode system that can align the capillary outlet with the working electrode without a three-dimensional micromanipulator. The five analytes could be well separated within 10 min in a 40 cm length capillary at a separation voltage of 9 kV in a 40 mmol/l borate buffer (pH 10.0) containing 100 mmol/l sodium dodecyl sulfate. Good linearity was observed between peak current and concentration of bases over three orders of magnitude with the detection limits (SIN=3) ranging from 1.28 x 10(-6) to 5.02 x 10(-6) mol/l. This proposed method demonstrated long-term stability and reproducibility with relative standard deviations of less than 5% for both migration time and peak current (n=7). It has been successfully applied to determine bases including 5-MC in the hydrolysates of fish sperm DNA, calf thymus DNA, and DNA isolated from spleen cells of female mice.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Chromatography, Micellar Electrokinetic Capillary / methods*
  • DNA / chemistry*
  • Electrochemistry
  • Purines / analysis*
  • Pyrimidines / analysis*
  • Reproducibility of Results
  • Sensitivity and Specificity

Substances

  • Purines
  • Pyrimidines
  • DNA