Trace level determination of organophosphorus pesticides in water with the new direct-electron ionization LC/MS interface

Anal Chem. 2002 Jul 15;74(14):3547-54. doi: 10.1021/ac015685f.

Abstract

A new LC/MS method for the determination of organophosphorus pesticides in water, based on the use of direct-electron ionization (EI) interface, is presented. Direct-EI is a new device that, in a very simple fashion, couples a nano-HPLC system with a mass spectrometer equipped with electron ionization capability. The nanoscale liquid flow allows for a direct introduction of eluate into the ion source and, after nebulization, for its ionization under typical EI conditions. Library-matchable EI spectra are generated for a choice of full scan or SIM detection of the analytes. In our case, a selection of organophosphorus pesticides, commonly distributed in local sugar beet cultivation, were considered. The new interface permits a very sensitive detection of the analytes in a wide range of linear response (0.09-9 ng). When applied to a real sample, the method allowed detecting four different pesticides at a concentration level of approximately 3 ng x L(-1).

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Chromatography, High Pressure Liquid / methods
  • Electrons
  • Insecticides / analysis*
  • Ions
  • Organothiophosphorus Compounds*
  • Spectrometry, Mass, Electrospray Ionization / methods*
  • Water Pollutants, Chemical / analysis*

Substances

  • Insecticides
  • Ions
  • Organothiophosphorus Compounds
  • Water Pollutants, Chemical