Synthetic hydraphile channels of appropriate length kill Escherichia coli

J Am Chem Soc. 2002 Aug 7;124(31):9022-3. doi: 10.1021/ja017052o.

Abstract

Crown ether-based synthetic cation conducting channels called hydraphiles show clear ionophoretic activity in phospholipid vesicles. These compounds are shown to be active against the bacterium E. coli. Disk diffusion assays were performed to assess the toxicity of different hydraphile derivatives. Liquid culture tests were conducted to quantitate the dependence of bacterical activity on channel length. It is proposed that hydraphiles are toxic to bacteria as a result of channel formation in the membrane. The bactericidal activity is found to depend at least on the presence of a functional central relay and proper channel length. It is speculated that hydraphiles insert into the bilayer and disrupt the cell's osmotic balance, leading to cell death.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Ampicillin Resistance
  • Escherichia coli / drug effects*
  • Indicators and Reagents
  • Ion Channels / chemistry
  • Ion Channels / pharmacology*
  • Iontophoresis
  • Lipid Bilayers
  • Magnetic Resonance Spectroscopy
  • Microbial Sensitivity Tests
  • Microscopy, Fluorescence
  • Phospholipids
  • Sodium / metabolism

Substances

  • Indicators and Reagents
  • Ion Channels
  • Lipid Bilayers
  • Phospholipids
  • Sodium