A potent analog of 1alpha,25-dihydroxyvitamin D3 selectively induces bone formation

Proc Natl Acad Sci U S A. 2002 Oct 15;99(21):13487-91. doi: 10.1073/pnas.202471299. Epub 2002 Oct 8.

Abstract

1,25-Dihydroxyvitamin D(3) [1,25(OH)(2)D(3)] is a principal regulator of calcium and phosphorus homeostasis through actions on intestine, kidney, and bone. 1,25(OH)(2)D(3) is not considered to play a significant role in bone formation, except for its role in supporting mineralization. We report here on the properties of 2-methylene-19-nor-(20S)-1alpha,25(OH)(2)D(3) (2MD), a highly potent analog of 1,25(OH)(2)D(3) that induces bone formation both in vitro and in vivo. Selectivity for bone was first demonstrated through the observation that 2MD is at least 30-fold more effective than 1,25(OH)(2)D(3) in stimulating osteoblast-mediated bone calcium mobilization while being only slightly more potent in supporting intestinal calcium transport. 2MD is also highly potent in promoting osteoblast-mediated osteoclast formation in vitro, a process essential to both bone resorption and formation. Most significantly, 2MD at concentrations as low as 10(-12) M causes primary cultures of osteoblasts to produce bone in vitro. This effect is not found with 1,25(OH)(2)D(3) even at 10(-8) M, suggesting that 2MD might be osteogenic in vivo. Indeed, 2MD (7 pmol/day) causes a substantial increase (9%) in total body bone mass in ovariectomized rats over a 23-week period. 1,25(OH)(2)D(3) (500 pmol three times a week) only prevented the bone loss associated with ovariectomy and did not increase bone mass. These results indicate that 2MD is a potent bone-selective analog of 1,25(OH)(2)D(3) potentially effective in treating bone loss diseases.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Animals
  • Bone Density / drug effects
  • Bone and Bones / drug effects
  • Bone and Bones / metabolism
  • Calcitriol / analogs & derivatives*
  • Calcitriol / pharmacology*
  • Calcium / metabolism
  • Carrier Proteins / metabolism
  • Cells, Cultured
  • Female
  • Humans
  • In Vitro Techniques
  • Intestinal Mucosa / metabolism
  • Intestines / drug effects
  • Male
  • Membrane Glycoproteins / metabolism
  • Osteoclasts / cytology
  • Osteoclasts / drug effects
  • Osteogenesis / drug effects*
  • Ovariectomy
  • RANK Ligand
  • Rats
  • Rats, Sprague-Dawley
  • Receptor Activator of Nuclear Factor-kappa B
  • Receptors, Calcitriol / drug effects
  • Receptors, Calcitriol / metabolism

Substances

  • 2-methylene-1,25-dihydroxy-19-norvitamin D3
  • Carrier Proteins
  • Membrane Glycoproteins
  • RANK Ligand
  • Receptor Activator of Nuclear Factor-kappa B
  • Receptors, Calcitriol
  • TNFRSF11A protein, human
  • TNFSF11 protein, human
  • Calcitriol
  • Calcium