Crystallization and preliminary X-ray crystallographic studies of 3-deoxy-manno-octulosonate cytidylyltransferase from Haemophilus influenzae

Acta Crystallogr D Biol Crystallogr. 2003 Jan;59(Pt 1):180-2. doi: 10.1107/s0907444902019698. Epub 2002 Dec 19.

Abstract

The enzyme 3-deoxy-manno-octulosonate cytidylyltransferase (CMP-KDO synthetase; CKS) catalyzes the activation of 3-deoxy-manno-octulosonate (KDO) by forming CMP-KDO. It is essential for the biosynthesis of lipopolysaccharides in Gram-negative bacteria and is a potential target for the discovery of antibacterial agents. L-CKS from Haemophilus influenzae was overexpressed with a C-terminal hexahistidine tag in Escherichia coli and crystallized in the presence of the substrate KDO at 297 K using PEG 4000 as a precipitant and ethylene glycol as an additive. The diffraction limit and spot shape of the native crystal could be improved significantly by dehydration/annealing. X-ray diffraction data were collected to 2.5 A resolution from a native crystal. The crystals are orthorhombic, belonging to the space group P2(1)2(1)2(1), with unit-cell parameters a = 48.6, b = 83.1, c = 117.3 A. The presence of two monomers of recombinant L-CKS in the crystallographic asymmetric unit gives a reasonable V(M) of 2.05 A(3) Da(-1), with a solvent content of 40.0%.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Crystallization
  • Crystallography, X-Ray / methods
  • DNA Primers / genetics
  • Escherichia coli / enzymology
  • Escherichia coli / genetics
  • Haemophilus influenzae / enzymology*
  • Haemophilus influenzae / genetics
  • Nucleotidyltransferases / chemistry*
  • Nucleotidyltransferases / genetics
  • Nucleotidyltransferases / metabolism
  • Recombinant Proteins / chemistry
  • Recombinant Proteins / genetics
  • Recombinant Proteins / metabolism
  • Sugar Acids / metabolism
  • Water / chemistry

Substances

  • DNA Primers
  • Recombinant Proteins
  • Sugar Acids
  • Water
  • 2-keto-3-deoxyoctonate
  • Nucleotidyltransferases
  • 3-deoxy-manno-octulosonate cytidyltransferase

Associated data

  • PDB/1HE7