Supercritical extraction of essential oil from aniseed (Pimpinella anisum L) using CO2: solubility, kinetics, and composition data

J Agric Food Chem. 2003 Mar 12;51(6):1518-23. doi: 10.1021/jf0257493.

Abstract

Supercritical fluid extraction (SFE) from aniseed using carbon dioxide was performed at 30 degrees C and pressures of 80-180 bar. The chemical composition of the SFE extract was determined by GC-MS; the quantitative analysis was done by GC-FID and TLC. The total amount of extractable substances or global yield (mass of extract/mass of feed) for the SFE process varied from 3.13 to 10.67% (mass). The solubilities of the anise essential oil in CO(2) were 0.0110, 0.0277, 0.0143, and 0.0182 kg of solute/kg of CO(2) at 80, 100, 140, and 180 bar, respectively. The major compounds identified and quantified in the extracts were anethole ( approximately 90%), gamma-himachalene (2-4%), p-anisaldehyde (<1%), methylchavicol (0.9-1.5%), cis-pseudoisoeugenyl 2-methylbutyrate ( approximately 3%), and trans-pseudoisoeugenyl 2-methylbutyrate ( approximately 1.3%). The Sovová model described quite well the experimental overall extraction curves.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Carbon Dioxide
  • Chromatography, Supercritical Fluid / methods*
  • Chromatography, Thin Layer
  • Gas Chromatography-Mass Spectrometry
  • Kinetics
  • Oils, Volatile / chemistry*
  • Pimpinella / chemistry*
  • Solubility

Substances

  • Oils, Volatile
  • Carbon Dioxide