Apoptotic cell death induction by F 11782 a novel dual catalytic inhibitor of topoisomerases I and II

Biochem Pharmacol. 2003 Mar 1;65(5):755-63. doi: 10.1016/s0006-2952(02)01564-2.

Abstract

F 11782 (2",3"-bis-pentafluorophenoxyacetyl-4",6"ethylidene-beta-D-glucoside of 4'-phosphate-4'-dimethylepipodophyllotoxin-2N-methyl glucamine salt), is a novel dual catalytic inhibitor of topoisomerases I and II characterised by marked in vivo antitumour activity, which also proved cytotoxic and exhibited DNA damaging properties in vitro. Mechanisms associated with this cell killing by F 11782 have been examined in P388 leukaemia cells. Treatment with F 11782 resulted in a dose-dependent DNA fragmentation coupled with the characteristic morphological features of apoptosis. Apoptosis-inducing concentrations of F 11782 induced caspases-3/7 activation accompanied by proteolytic cleavage of poly(ADP-ribose)-polymerase, which could be inhibited by the caspase inhibitor acetyl-Asp-Glu-Val-Asp-aldehyde. In addition, F 11782-induced apoptosis in P388 cells was associated with an increased expression of the pro-apototic Bax protein, without significant changes in the level of the anti-apoptotic Bcl-2 protein, and with modification at the mitochondrial membrane function. These results indicate that F 11782 leads to apoptosis through a caspase-3/7 dependent mechanism and suggest that the so-called "mitochondrial pathway" is implicated in F 11782-induced apoptosis in P388 cells.

MeSH terms

  • Animals
  • Apoptosis*
  • Caspases / metabolism
  • Catalytic Domain
  • Cell Cycle / drug effects
  • Cell Division / drug effects
  • Cell Size / drug effects
  • DNA Fragmentation / drug effects
  • Gene Expression / drug effects
  • Leukemia P388 / pathology
  • Membrane Potentials / drug effects
  • Mice
  • Mitochondria / drug effects
  • Mitochondria / physiology
  • Naphthalenes / pharmacology*
  • Poly(ADP-ribose) Polymerases / metabolism
  • Proto-Oncogene Proteins / biosynthesis
  • Proto-Oncogene Proteins c-bcl-2 / biosynthesis
  • Pyrans / pharmacology*
  • Topoisomerase I Inhibitors*
  • Topoisomerase II Inhibitors*
  • Tumor Cells, Cultured
  • bcl-2-Associated X Protein

Substances

  • Bax protein, mouse
  • Naphthalenes
  • Proto-Oncogene Proteins
  • Proto-Oncogene Proteins c-bcl-2
  • Pyrans
  • Topoisomerase I Inhibitors
  • Topoisomerase II Inhibitors
  • bcl-2-Associated X Protein
  • Poly(ADP-ribose) Polymerases
  • Caspases
  • tafluposide