TH1 and TH2 cytokine inhibition by 3,5-bis(trifluoromethyl)pyrazoles, a novel class of immunomodulators

Cell Immunol. 2002 Dec;220(2):134-42. doi: 10.1016/s0008-8749(03)00005-4.

Abstract

In order to discover novel immunomodulators for application in treating autoimmune diseases, a stable Jurkat transfectant was constructed in which luciferase reporter gene is driven by a full-length IL-2 promotor. A chemical library was screened to identify compounds that inhibited luciferase expression in Jurkat transfectants stimulated with PMA and ionomycin. A class of compounds (bis-trifluoromethyl pyrazole, BTPs) was identified from this screen. BTPs were shown to inhibit anti-CD3 and anti-CD28 antibody-induced IL-2 secretion, mixed lymphocyte reaction, and Con A-induced T cell proliferation in normal human peripheral blood T cells. In addition, mRNA levels of IL-4, IL-5, IL-9, IL-10, IL-13, IL-15, and IFN-gamma were markedly inhibited by BTPs in peripheral blood mononuclear cells stimulated by Con A as determined by multi-probe RNA protection assay. Furthermore, IL-2, IL-4, IL-5, and IFN-gamma secretion by Hut 78 cells or CD3(+) T cells stimulated with PMA plus ionomycin or anti-CD3 antibody plus PMA were inhibited in a concentration-dependent manner by BTPs. Therefore, BTPs inhibit a wide spectrum of cytokine production including TH1 and TH2 type cytokines. Taken together, these compounds may be useful for treating autoimmune diseases and organ transplant rejection.

MeSH terms

  • Adjuvants, Immunologic / pharmacology*
  • Calcium / immunology
  • Cell Division / immunology
  • Concanavalin A / immunology
  • Cytokines / antagonists & inhibitors*
  • Cytokines / biosynthesis
  • Cytokines / genetics
  • Cytokines / immunology
  • Humans
  • Interleukin-2 / immunology
  • Ionomycin / immunology
  • Ionophores / immunology
  • Jurkat Cells / immunology
  • Lymphocyte Activation / drug effects
  • Lymphocyte Activation / immunology
  • Lymphocyte Culture Test, Mixed
  • Promoter Regions, Genetic / immunology
  • Pyrazoles / pharmacology*
  • RNA / genetics
  • RNA / immunology
  • Tetradecanoylphorbol Acetate / immunology
  • Th1 Cells / drug effects*
  • Th1 Cells / immunology
  • Th1 Cells / metabolism
  • Th2 Cells / drug effects*
  • Th2 Cells / immunology
  • Th2 Cells / metabolism
  • Transfection

Substances

  • Adjuvants, Immunologic
  • Cytokines
  • Interleukin-2
  • Ionophores
  • Pyrazoles
  • Concanavalin A
  • Ionomycin
  • RNA
  • Tetradecanoylphorbol Acetate
  • Calcium