Effects of phenyl N-tert-butyl nitrone and its derivatives on the early phase of hepatocarcinogenesis in rats fed a choline-deficient, L-amino acid-defined diet

Cancer Sci. 2003 Jan;94(1):26-31. doi: 10.1111/j.1349-7006.2003.tb01347.x.

Abstract

The present study examined the effects of various derivatives of a radical trapping agent, phenyl N-tert-butyl nitrone, on the early phase of hepatocarcinogenesis in male Wistar rats fed a choline-deficient, L-amino acid-defined diet for 16 weeks. The derivatives used were 4-hydroxyphenyl (a physiologically major metabolite), 3-hydroxyphenyl, 2-hydroxyphenyl and 2-sulfoxyphenyl N-tert-butyl nitrone, and their effects were studied in a comparison with those of the parent compound, phenyl N-tert-butyl nitrone. The sizes of putatively preneoplastic, glutathione S-transferase placental form-positive lesions and the levels of extra-nuclear oxidative injury of hepatocytes, using the formation of 2-thiobarbituric acid-reacting substances as a parameter, were decreased by all doses (0.009%, 0.045% and 0.090% in diet) of 4-hydroxyphenyl N-tert-butyl nitrone and only by the highest dose of 3-hydroxyphenyl N-tert-butyl nitrone and phenyl N-tert-butyl nitrone. While 4-hydroxyphenyl N-tert-butyl nitrone, 3-hydroxyphenyl N-tert-butyl nitrone and phenyl N-tert-butyl nitrone all enhanced and inhibited hepatocellular apoptosis in preneoplastic lesions and their surrounding tissue, respectively, only 4-hydroxyphenyl N-tert-butyl nitrone additionally inhibited hepatocyte proliferation both in preneoplastic lesions and their surrounding tissue. 2-Hydroxyphenyl or 2-sulfoxyphenyl N-tert-butyl nitrone did not exert any of the above effects. These results suggest that the selective induction of apoptosis in preneoplastic hepatocyte populations plays a crucial role in the inhibition of hepatocarcinogenesis derived by phenyl N-tert-butyl nitrone and its effective derivatives. Further, the metabolic conversion to 4-hydroxyphenyl N-tert-butyl nitrone may also be important for the inhibitory effects of phenyl N-tert-butyl nitrone on hepatocarcinogenesis.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Amino Acids / administration & dosage*
  • Animals
  • Anticarcinogenic Agents / pharmacology
  • Anticarcinogenic Agents / therapeutic use*
  • Apoptosis / drug effects
  • Biomarkers, Tumor / analysis
  • Cell Division / drug effects
  • Choline Deficiency / complications*
  • Cyclic N-Oxides
  • Dose-Response Relationship, Drug
  • Fatty Liver / drug therapy
  • Fatty Liver / etiology
  • Free Radical Scavengers / pharmacology
  • Free Radical Scavengers / therapeutic use*
  • Glutathione Transferase / analysis
  • Hepatocytes / drug effects
  • Hepatocytes / enzymology
  • Liver Cirrhosis / drug therapy
  • Liver Cirrhosis / etiology
  • Liver Neoplasms, Experimental / enzymology
  • Liver Neoplasms, Experimental / etiology
  • Liver Neoplasms, Experimental / prevention & control*
  • Male
  • Molecular Structure
  • Nitrogen Oxides / pharmacology
  • Nitrogen Oxides / therapeutic use*
  • Oxidative Stress
  • Precancerous Conditions / drug therapy
  • Precancerous Conditions / enzymology
  • Precancerous Conditions / pathology
  • Rats
  • Rats, Wistar

Substances

  • Amino Acids
  • Anticarcinogenic Agents
  • Biomarkers, Tumor
  • Cyclic N-Oxides
  • Free Radical Scavengers
  • Nitrogen Oxides
  • phenyl-N-tert-butylnitrone
  • Glutathione Transferase