Synthesis and activity of a C-8 keto pleuromutilin derivative

Bioorg Med Chem Lett. 2003 May 19;13(10):1751-3. doi: 10.1016/s0960-894x(03)00297-x.

Abstract

A C-8 keto pleuromutilin derivative has been synthesized from the biotransformation product 8-hydroxy mutilin. A key step in the process was the selective oxidation at C-8 of 8-hydroxy mutilin using tetrapropylammonium perruthenate. The presence of the C-8 keto group precipitated interesting intramolecular chemistry to afford a compound (10) with a novel pleuromutilin-derived ring system.

MeSH terms

  • Biotransformation
  • Diterpenes / chemical synthesis*
  • Ketones / chemistry
  • Oxidation-Reduction
  • Pleuromutilins
  • Polycyclic Compounds / chemistry

Substances

  • Diterpenes
  • Ketones
  • Polycyclic Compounds
  • mutilin