Dihydrochalcones: evaluation as novel radical scavenging antioxidants

J Agric Food Chem. 2003 May 21;51(11):3309-12. doi: 10.1021/jf0341060.

Abstract

Dihydrochalcones are a family of bicyclic flavonoids, defined by the presence of two benzene rings joined by a saturated three carbon bridge. In the present study, we systematically examined the antioxidant activities of dihydrochalcones against the stable free radical (1,1-diphenyl-2-picrylhydrazyl) and lipid peroxidation in the erythrocyte membrane. All dihydrochalcones exhibited higher antioxidant activities than the corresponding flavanones. The (1)H NMR analysis indicated that the active dihydrochalcone has a time-averaged conformation in which the aromatic A ring is orthogonal to the carbonyl group, while the inactive dihydrochalcone such as 2'-O-methyl-phloretin has a strongly hydrogen-bonded phenolic hydroxyl group, suggestive of a coplanar conformation. A hydroxyl group at the 2'-position of the dihydrochalcone A ring, newly formed by reduction of the flavanone C ring, is an essential pharmacophore for its radical scavenging potential.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Antioxidants / pharmacology*
  • Biphenyl Compounds
  • Chalcone / analogs & derivatives*
  • Chalcone / chemistry
  • Chalcone / pharmacology*
  • Chalcones
  • Erythrocyte Membrane / chemistry
  • Flavanones*
  • Flavonoids / pharmacology
  • Free Radical Scavengers / pharmacology*
  • Hydrogen Bonding
  • Hydroxylation
  • Lipid Peroxidation / drug effects
  • Magnetic Resonance Spectroscopy
  • Molecular Structure
  • Picrates / chemistry
  • Structure-Activity Relationship

Substances

  • Antioxidants
  • Biphenyl Compounds
  • Chalcones
  • Flavanones
  • Flavonoids
  • Free Radical Scavengers
  • Picrates
  • Chalcone
  • 1,1-diphenyl-2-picrylhydrazyl
  • dihydrochalcone
  • flavanone