A new method for the stereoselective synthesis of alpha-substituted serine amino acid analogues

Org Lett. 2003 Oct 30;5(22):4017-20. doi: 10.1021/ol034984j.

Abstract

[reaction: see text]. A new method was developed for the stereoselective synthesis of alpha-substituted serine amino acids. The strategy utilizes a common enantiomerically enriched intermediate obtained through an enzymatic desymmetrization. A variety of amino acids were synthesized in good ee's through nucleophilic acetylide addition reactions and palladium-catalyzed Sonogashira couplings.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Catalysis
  • Chemistry, Organic / methods*
  • Molecular Structure
  • Palladium / chemistry
  • Serine / analogs & derivatives*
  • Serine / chemical synthesis*
  • Serine / chemistry
  • Stereoisomerism

Substances

  • Serine
  • Palladium