Proteomic analysis of the benzoate degradation pathway in Acinetobacter sp. KS-1

Res Microbiol. 2003 Dec;154(10):697-703. doi: 10.1016/j.resmic.2003.09.003.

Abstract

The purpose of this study was to perform proteome analysis of Acinetobacter sp. KS-1, a bacterium capable of degrading benzoate as a sole carbon source. In order to understand the benzoate degradation pathway used by strain KS-1, proteomes of benzoate-cultured and succinate-cultured KS-1 were comparatively analyzed by two dimensional gel electrophoresis (2-DE). Eighteen protein spots proteins were exclusively induced from the benzoate-cultured strain KS-1. Of these 18 spots, two benzoate-degrading enzymes (catechol 1,2-dioxygenase and beta-ketoadipate succinyl-CoA transferase) were identified by MS/MS analysis by MALDI-TOF/TOF mass spectrometry, which suggests that strain KS-1 degrades benzoate by the beta-ketoadipate pathway. DEAE-chromatography suggested that strain KS-1 induced only one type of catechol 1,2-dioxygenase during benzoate degradation. The catechol 1,2-dioxygenase was purified using three steps of ammonium sulfate precipitation, DEAE-sepharose, and Mono-Q chromatography. The purified catechol 1,2-dioxygenase of strain KS-1 had strong dioxygenase activity for 4-methylcatechol as well as catechol. Sequencing analysis using N-terminal and internal amino acid sequences showed that this catechol 1,2-dioxygenase is highly homologous with catechol 1,2-dioxygenase of Acinetobacter radioresistens. These results suggest that comparative proteomic analysis of biodegrading bacteria cultured under different conditions may be a useful initial step toward the elucidation of the aromatic compound degradation pathway.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Acinetobacter / genetics
  • Acinetobacter / growth & development
  • Acinetobacter / metabolism*
  • Amino Acid Sequence
  • Bacterial Proteins / chemistry
  • Bacterial Proteins / genetics
  • Bacterial Proteins / metabolism*
  • Benzoates / metabolism*
  • Biodegradation, Environmental
  • Catechol 1,2-Dioxygenase
  • Dioxygenases*
  • Electrophoresis, Gel, Two-Dimensional
  • Molecular Sequence Data
  • Oxygenases / chemistry
  • Oxygenases / genetics
  • Oxygenases / isolation & purification
  • Oxygenases / metabolism
  • Peptides / chemistry
  • Proteome*
  • Sequence Analysis, DNA
  • Succinic Acid / metabolism

Substances

  • Bacterial Proteins
  • Benzoates
  • Peptides
  • Proteome
  • Succinic Acid
  • Oxygenases
  • Dioxygenases
  • Catechol 1,2-Dioxygenase