The nature of oxygen exchange in ZrW2O8 revealed by two-dimensional solid-state 17O NMR

Chem Commun (Camb). 2004 Feb 21:(4):392-3. doi: 10.1039/b314076h. Epub 2004 Jan 23.

Abstract

17O magic angle spinning (MAS) NMR has been used to determine the nature of oxygen exchange in ZrW(2)O(8). A highly effective isotopic labelling technique has been developed and 1D NMR and 2D exchange spectroscopy (EXSY) experiments have revealed that mutual exchange occurs between all oxygen sites, even at temperatures considerably below the alpha to beta order-disorder phase transition.