Parallel substrate binding sites in a beta-agarase suggest a novel mode of action on double-helical agarose

Structure. 2004 Apr;12(4):623-32. doi: 10.1016/j.str.2004.02.020.

Abstract

Agarose is a gel-forming polysaccharide with an alpha-L(1,4)-3,6-anhydro-galactose, beta-D(1,3)-galactose repeat unit, from the cell walls of marine red algae. beta-agarase A, from the Gram-negative bacterium Zobellia galactanivorans, is secreted to the external medium and degrades agarose with an endo-mechanism. The structure of the inactive mutant beta-agarase A-E147S in complex with agaro-octaose has been solved at 1.7 A resolution. Two oligosaccharide chains are bound to the protein. The first one resides in the active site channel, spanning subsites -4 to -1. A second oligosaccharide binding site, on the opposite side of the protein, was filled with eight sugar units, parallel to the active site. The crystal structure of the beta-agarase A with agaro-octaose provides detailed information on agarose recognition in the catalytic site. The presence of the second, parallel, binding site suggests that the enzyme might be able to unwind the double-helical structure of agarose prior to the catalytic cleavage.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Binding Sites
  • Catalytic Domain
  • Crystallization
  • Glycoside Hydrolases / chemistry*
  • Glycoside Hydrolases / metabolism
  • Gram-Negative Bacteria / enzymology
  • Gram-Negative Bacteria / metabolism
  • Protein Binding
  • Protein Structure, Tertiary
  • Sepharose / metabolism*

Substances

  • Sepharose
  • Glycoside Hydrolases
  • agarase

Associated data

  • PDB/1URX