Photocatalytic degradation of methyl-red by immobilised nanoparticles of TiO2 and ZnO

Water Sci Technol. 2004;49(4):183-8.

Abstract

In this work, we report on the degradation of methyl-red (2-(4-Dimethylamino-phenylazo)-benzoic acid--C.I. 13020) under UV irradiation in the presence of nanosized ZnO and TiO2. Oxide nanocrystals with controlled size were synthesised by using non-hydrolytic approaches and tested for the photocatalysed degradation. The performances of the immobilised nanoparticles were compared with their commercial counterparts after immobilization onto a solid support. The influence of some experimental conditions, namely pH and dye concentration, were investigated by monitoring the dye decoloration spectrophotometrically. Several intermediate by-products were identified by HPLC-MS, showing that two different mechanisms were operative during the photocatalytic oxidation.

MeSH terms

  • Catalysis
  • Chromatography, High Pressure Liquid
  • Colloids
  • Coloring Agents / chemistry*
  • Mass Spectrometry
  • Nanotechnology*
  • Particle Size
  • Photochemistry
  • Titanium / chemistry*
  • Water Pollutants / isolation & purification*
  • Water Purification / methods*
  • p-Dimethylaminoazobenzene / analogs & derivatives
  • p-Dimethylaminoazobenzene / chemistry*
  • p-Dimethylaminoazobenzene / isolation & purification*

Substances

  • Colloids
  • Coloring Agents
  • Water Pollutants
  • methyl-red (2-(4-dimethylamino-phenylazo)-benzoic acid)
  • titanium dioxide
  • p-Dimethylaminoazobenzene
  • Titanium