Synthesis of marimastat and a marimastat conjugate for affinity chromatography and surface plasmon resonance studies

Bioconjug Chem. 2004 May-Jun;15(3):594-600. doi: 10.1021/bc034225l.

Abstract

Immobilized small-molecule inhibitors are suited for enrichment of biomolecules by affinity chromatography, as it is shown for metalloproteinases and an immobilizable derivative of the hydroxamate-type inhibitor marimastat. A new asymmetric synthesis of marimastat is presented that allows for site-specific attachment to a solid surface, e.g., a chromatography matrix or a surface plasmon resonance sensor chip. The latter technique is shown to be a valuable tool for the optimization of binding and elution conditons of biomolecules in affinity chromatography.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biosensing Techniques / methods*
  • Chromatography, Affinity / methods
  • Hydroxamic Acids* / chemical synthesis
  • Hydroxamic Acids* / chemistry
  • Molecular Structure
  • Surface Plasmon Resonance / methods*
  • Time Factors

Substances

  • Hydroxamic Acids
  • marimastat