Retinoic acid can be produced from excentric cleavage of beta-carotene in human intestinal mucosa

Arch Biochem Biophys. 1992 Mar;293(2):298-304. doi: 10.1016/0003-9861(92)90399-h.

Abstract

The hypothesis that retinoic acid (RA) is produced from the excentric cleavage of beta-carotene was tested in human intestinal homogenates in vitro. Significant amounts of RA were identified by HPLC and derivatization after incubation of intestinal mucosal homogenates with retinal, beta-carotene, or beta-apocarotenals at 37 degrees C for 60 min. RA formation was inhibited, in a dose-dependent fashion, when retinal was incubated in the presence of 0.1-3.0 mM citral (3,7-dimethyl-2,6-octadienal) under identical experimental conditions. The formation of RA from both beta-carotene and beta-apocarotenals was dose and time dependent and RA was the major metabolite of both beta-apo-8'-carotenal and beta-apo-12'-carotenal after the incubation. However, citral (0.1 to 4 mM) did not inhibit the formation of beta-apocarotenals and RA from 2 microM beta-carotene (P greater than 0.05), which proves the existence of an excentric cleavage mechanism for beta-carotene conversion into retinoids. Furthermore, RA formation from both beta-apo-8'-carotenal and beta-apo-12'-carotenal in human intestinal homogenate occurred in the presence of citral, which demonstrates that RA can be produced from excentric cleavage of beta-carotene via a series of beta-apocarotenals as intermediates.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Acyclic Monoterpenes
  • Binding, Competitive
  • Carotenoids / chemistry
  • Carotenoids / metabolism*
  • Humans
  • Hydrolysis
  • In Vitro Techniques
  • Intestinal Mucosa / chemistry
  • Intestinal Mucosa / metabolism*
  • Monoterpenes*
  • Terpenes / pharmacology
  • Tretinoin / antagonists & inhibitors
  • Tretinoin / chemistry
  • Tretinoin / metabolism*
  • beta Carotene

Substances

  • Acyclic Monoterpenes
  • Monoterpenes
  • Terpenes
  • beta Carotene
  • Carotenoids
  • Tretinoin
  • citral