Identification of glutathione-derived metabolites from an IP receptor antagonist

Drug Metab Dispos. 2004 Dec;32(12):1482-90. doi: 10.1124/dmd.104.000471. Epub 2004 Sep 15.

Abstract

The metabolic fate of three aromatic carboxylic acid analogs under evaluation as prostaglandin I2-preferring receptor antagonists was studied. The initial analog with unsubstituted phenyl groups was subject to a complex set of aromatic oxidative biotransformations. By introduction of one or two fluorines, these pathways were inhibited. All three analogs were metabolized to a wide variety of carboxylic acid conjugates. Among these were several conjugates formed via secondary metabolism and oxidation of acyl glutathione intermediates. Two of the structure classes, represented by the S-methyl-N-cysteinylglycine conjugate and the N-cysteinylglycine disulfide conjugates, have been described only rarely in the literature. The related S-oxide of the S-methyl-N-cysteinylglycine conjugate and the N,S-bis-acyl derivative of cysteinylglycine are here described for the first time as conjugate metabolites of carboxylic drugs.

MeSH terms

  • Animals
  • Biotransformation
  • Chromatography, High Pressure Liquid
  • Dogs
  • Epoprostenol / metabolism*
  • Glutathione / metabolism*
  • Haplorhini
  • Hepatocytes / metabolism
  • In Vitro Techniques
  • Indicators and Reagents
  • Isotope Labeling
  • Liver / metabolism
  • Magnetic Resonance Spectroscopy
  • Molecular Weight
  • Oxidation-Reduction
  • Perfusion
  • Rats
  • Receptors, Epoprostenol / antagonists & inhibitors*
  • Spectrometry, Mass, Electrospray Ionization
  • Spectrophotometry, Ultraviolet

Substances

  • Indicators and Reagents
  • Receptors, Epoprostenol
  • Epoprostenol
  • Glutathione