Alkyl lysophosphatidic acid and fluoromethylene phosphonate analogs as metabolically-stabilized agonists for LPA receptors

Bioorg Med Chem Lett. 2004 Nov 1;14(21):5323-8. doi: 10.1016/j.bmcl.2004.08.019.

Abstract

We describe an efficient method for the synthesis of alkyl lysophosphatidic acid (LPA) analogs as well as alkyl LPA mono- and difluoromethylene phosphonate analogs. Each alkyl LPA analog was evaluated for subtype-specific LPA receptor agonist activity using a cell migration assay for LPA(1) activation in cancer cells and an intracellular calcium mobilization assay for LPA(2) and LPA(3) activation. Alkyl LPAs induced pronounced cell migration activity with equivalent or higher potency than sn-1-oleoyl LPA, while the alkyl LPA fluoromethylene phosphonates proved to be less potent agonists in this assay. However, each alkyl LPA analog activated Ca(2+) release by activation of LPA(2) and LPA(3) receptors. Interestingly, the absolute configuration of the sn-2 hydroxyl group of the alkyl LPA analogs was not recognized by any of the three LPA receptors. The use of alkyl LPA analogs further expands the scope of structure-activity studies, which will better define LPA-LPA receptor interactions.

Publication types

  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, P.H.S.

MeSH terms

  • Animals
  • Antineoplastic Agents / chemical synthesis*
  • Antineoplastic Agents / chemistry
  • Antineoplastic Agents / pharmacology
  • Calcium / metabolism
  • Cell Line, Tumor
  • Cell Movement / drug effects
  • Humans
  • Insecta
  • Intracellular Fluid / metabolism
  • Lysophospholipids / chemical synthesis*
  • Lysophospholipids / chemistry
  • Lysophospholipids / pharmacology
  • Molecular Conformation
  • Organophosphonates / chemical synthesis*
  • Organophosphonates / chemistry
  • Organophosphonates / pharmacology
  • Protein Isoforms / agonists
  • Receptors, Lysophosphatidic Acid / agonists*
  • Structure-Activity Relationship
  • Substrate Specificity

Substances

  • Antineoplastic Agents
  • Lysophospholipids
  • Organophosphonates
  • Protein Isoforms
  • Receptors, Lysophosphatidic Acid
  • lysophosphatidic acid
  • Calcium