Enhancement of the efficacy of an antagonist of an extracellular receptor by attachment to the surface of a biocompatible carrier

Pharm Res. 2004 Oct;21(10):1880-5. doi: 10.1023/b:pham.0000045243.98010.b6.

Abstract

Purpose: In order to improve the in vitro and in vivo efficacy of an integrin antagonist (IA) of the extracellular domain of the alphavbeta3 integrin, a receptor upregulated on tumor neovasculature, the IA was attached to the surface of a dextran-coated liposome (DCL). IA-DCLs were characterized in vitro, and the pharmacokinetic and antitumor properties were assessed in vivo.

Methods: The in vitro binding properties were measured with purified integrin, endothelial cells, and melanoma cells. The pharmacokinetic parameters were measured in healthy mice with 14C-labeled IA-DCLs and anti-tumor efficacy was assessed with the M21 human melanoma xenograft mouse model.

Results: In vitro, IC50 values for IA-DCLs and IA are similar, and IA-DCLs inhibit cell proliferation relative to controls. IA-DCLs are stable in serum, and the pharmacokinetic half-life in mice is 23 h. In the M21/mouse model, statistically significant inhibition of tumor growth was observed for mice treated with IA-DCLs, whereas controls including saline, DCLs lacking IA, and cyclo(RGDfV) were ineffective. Increased apoptosis and a reduction in vessel counts relative to controls were present in tumors from animals treated with IA-DCLs.

Conclusions: These results demonstrate that IA-DCLs are potent anti-angiogenic therapeutic agents with superior in vivo activity and pharmacology compared to unmodified IA.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Angiogenesis Inhibitors / administration & dosage
  • Angiogenesis Inhibitors / pharmacology
  • Animals
  • Antineoplastic Agents / administration & dosage*
  • Antineoplastic Agents / pharmacokinetics
  • Antineoplastic Agents / pharmacology
  • Biocompatible Materials*
  • Cell Adhesion / drug effects
  • Cell Proliferation / drug effects
  • Dextrans
  • Drug Carriers
  • Drug Compounding
  • Drug Delivery Systems
  • Endothelial Cells / drug effects
  • Half-Life
  • Humans
  • In Situ Nick-End Labeling
  • Integrin alphaVbeta3 / antagonists & inhibitors*
  • Liposomes
  • Melanoma / drug therapy
  • Melanoma / pathology
  • Mice
  • Neoplasm Transplantation
  • Neoplasms, Experimental / drug therapy
  • Tissue Distribution

Substances

  • Angiogenesis Inhibitors
  • Antineoplastic Agents
  • Biocompatible Materials
  • Dextrans
  • Drug Carriers
  • Integrin alphaVbeta3
  • Liposomes