Expression of a wheat cytochrome P450 monooxygenase in yeast and its inhibition by glyphosate

Pest Manag Sci. 2005 Apr;61(4):402-6. doi: 10.1002/ps.969.

Abstract

Glyphosate is a non-selective herbicide which acts by inhibiting 5-enolpyruvylshikimate-3-phosphate synthase. Wheat cytochrome P450 monooxygenase specifically catalyzes the metabolism of some sulfonylurea herbicides such as chlorsulfuron and triasulfuron. Here we report that glyphosate is an inhibitor of a wheat cytochrome (CYP71C6v1), the cDNA of which was amplified by RT-PCR and heterologously expressed in yeast. The microsomal fractions derived from this strain had a Soret peak at 502 nm in the reduced carbon monoxide difference spectrum, which is a typical spectral characteristic. The addition of glyphosate to the microsomal protein resulted in a Type II spectrum indicative of binding via the nitrogen group to haem of cytochrome P450 as a sixth ligand. A spectral dissociation constant, K(s) of 70 micromol litre(-1) was observed and an IC50 of 11 micromol litre(-1) was found for glyphosate inhibition of CYP71C6v1 P450 activity.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Base Sequence
  • Cytochrome P-450 Enzyme Inhibitors*
  • Cytochrome P-450 Enzyme System / genetics
  • Cytochrome P-450 Enzyme System / metabolism
  • Gene Expression
  • Glycine / analogs & derivatives*
  • Glycine / pharmacology*
  • Glyphosate
  • Herbicides / pharmacology*
  • Molecular Sequence Data
  • Organisms, Genetically Modified
  • Plant Proteins / genetics
  • Plant Proteins / metabolism
  • Saccharomyces cerevisiae / genetics
  • Triticum / enzymology*
  • Triticum / genetics

Substances

  • Cytochrome P-450 Enzyme Inhibitors
  • Herbicides
  • Plant Proteins
  • Cytochrome P-450 Enzyme System
  • Glycine