Observation of intrinsic size effects in the optical response of individual gold nanoparticles

Nano Lett. 2005 Mar;5(3):515-8. doi: 10.1021/nl050062t.

Abstract

The photothermal heterodyne imaging method is used to study for the first time the absorption spectra of individual gold nanoparticles with diameters down to 5 nm. Intrinsic size effects that result in a broadening of the surface plasmon resonance are unambiguously observed. Dispersions in the peak energies and homogeneous widths of the single-particle resonances are revealed. The experimental results are analyzed within the frame of Mie theory.

Publication types

  • Comparative Study
  • Evaluation Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Gold / analysis
  • Gold / chemistry*
  • Hot Temperature
  • Light
  • Nanotechnology / methods
  • Nanotubes / analysis
  • Nanotubes / chemistry*
  • Nanotubes / ultrastructure*
  • Particle Size
  • Surface Plasmon Resonance / methods*

Substances

  • Gold