Substrate specificity and preference of Delta6-desaturase of Mucor rouxii

FEBS Lett. 2005 May 9;579(12):2744-8. doi: 10.1016/j.febslet.2005.04.010. Epub 2005 Apr 20.

Abstract

The Delta(6)-fatty acid desaturase is a key enzyme in the synthesis of an important fatty acid, gamma-linolenic acid. We have characterized, by heterologous expression in Saccharomyces cerevisiae, substrate specificity and preference of Delta(6)-desaturase of Mucor rouxii. Fatty acid supplementation was carried out based on the predicted enzyme topology, fatty acid phenotype and the corresponding metabolic pathway in M. rouxii. The enzyme has a broad substrate specificity as based on C15-C18. The result also supported classification of the M. rouxii Delta(6)-desaturase into a front-end desaturase. Interestingly, a relatively rare activity based on odd acyl chains and not described previously in other eukaryotic Delta(6)-desaturases was also observed.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Chromatography, Gas
  • DNA, Complementary
  • Fatty Acid Desaturases / chemistry
  • Fatty Acid Desaturases / genetics
  • Fatty Acid Desaturases / metabolism*
  • Fatty Acids / analysis
  • Fatty Acids / chemistry
  • Mass Spectrometry
  • Mucor / enzymology*
  • Mucor / growth & development
  • Phylogeny
  • Plasmids
  • Protein Structure, Tertiary
  • Saccharomyces cerevisiae / enzymology
  • Saccharomyces cerevisiae / growth & development
  • Substrate Specificity
  • gamma-Linolenic Acid / biosynthesis*

Substances

  • DNA, Complementary
  • Fatty Acids
  • gamma-Linolenic Acid
  • Fatty Acid Desaturases