Bicelle membranes and their use for hydrophobic peptide studies by circular dichroism and solid state NMR

Biochim Biophys Acta. 2005 Aug 5;1724(3):315-23. doi: 10.1016/j.bbagen.2005.04.026.

Abstract

Mixtures of dicaproyl- (DC), dimyristoyl- (DM) and 1-tetradecanoyl-2-biphenylbutanoyl-(TBB) phosphatidylcholine (PC) in water produce bicelle membranes that are oriented by magnetic fields. DMPC/DCPC systems orient such that their membrane plane is parallel to the magnetic field, whereas for TBBPC/DCPC, the plane is perpendicular to the field. Partial temperature-composition-hydration diagrams are established using solid-state 31P-NMR. DMPC/DCPC bicelles exist on a large range of composition but on a narrow temperature domain (25-45 degrees C). At converse, TBBPC/DCPC form bicelles on a narrow compositional range but over a large temperature span (10-70 degrees C). The TBBPC/DCPC bicelles are shown to be a very powerful potential tool to study the orientation of hydrophobic helices in membranes using wide line 15N-NMR. The DMPC/DCPC system that undergoes a micelle-to-bicelle transition on going from 10 degrees C to 40 degrees C may be used with circular dichroism to study the state of association of hydrophobic helices within the membrane. Results suggest that the transmembrane fragment of the neu/erbB-2 receptor is monomeric in micellar medium and dimeric/multimeric in bicelle membranes.

Publication types

  • Comparative Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Circular Dichroism*
  • Dimyristoylphosphatidylcholine
  • Hydrophobic and Hydrophilic Interactions*
  • Liposomes
  • Magnetic Resonance Spectroscopy*
  • Membranes, Artificial*
  • Micelles
  • Molecular Sequence Data
  • Nitrogen Isotopes
  • Peptide Fragments / chemistry*
  • Phosphatidylcholines
  • Phosphorus Isotopes
  • Receptor, ErbB-2 / chemistry
  • Temperature
  • Water

Substances

  • Liposomes
  • Membranes, Artificial
  • Micelles
  • Nitrogen Isotopes
  • Peptide Fragments
  • Phosphatidylcholines
  • Phosphorus Isotopes
  • Water
  • 1,2-didecanoylphosphatidylcholine
  • Receptor, ErbB-2
  • Dimyristoylphosphatidylcholine