Photodynamic effects of a novel pterin derivative on a pancreatic cancer cell line

Biochem Biophys Res Commun. 2005 Aug 5;333(3):763-7. doi: 10.1016/j.bbrc.2005.05.185.

Abstract

6-Formylpterin (6FP) has the potential to produce singlet oxygen (1O2) under UV-A radiation. In order to apply this potential to anti-cancer photodynamic therapy (PDT), we prepared a novel variant of 6FP, 2-(N,N-dimethylaminomethyleneamino)-6-formyl-3-pivaloylpteridine-4-one (6FP-tBu-DMF), and examined its photodynamic effects on a pancreatic cancer cell line, Panc-1 cells. The study using laser scanning confocal microscopy showed that the drug uptake, the 1O2 generation, and cell death were observed in the 6FP-tBu-DMF-treated cells, while these phenomena were not observed in the 6FP-treated cells. The MTT assay also showed the decrease in cell viability only in the 6FP-tBu-DMF-treated cells. Since 6FP and 6FP-tBu-DMF generate 1O2 to the same extent under UV-A radiation in aqueous solutions, these results indicated that the differences in the photodynamic effects between 6FP and 6FP-tBu-DMF were entirely attributed to the differences in the cell permeability between them. The development of cell permeable pterin derivatives has the potential for application in PDT.

MeSH terms

  • Cell Line, Tumor
  • Electron Spin Resonance Spectroscopy
  • Humans
  • Microscopy, Confocal
  • Pancreatic Neoplasms / drug therapy*
  • Pancreatic Neoplasms / pathology
  • Photochemotherapy*
  • Pteridines / therapeutic use*

Substances

  • 2-(N,N-dimethylaminomethyleneamino)-6-formyl-3-pivaloylpteridin-4-one
  • Pteridines