Purification and characterization of a beta-D-mannosidase from the marine anaspidean Aplysia fasciata

J Biotechnol. 2005 Sep 22;119(1):26-35. doi: 10.1016/j.jbiotec.2005.06.003.

Abstract

A beta-D-mannosidase was purified to homogeneity from visceral mass extract of Aplysia fasciata a mollusc belonging to the order Anaspidea. The purified enzyme is a homodimer with a subunit mass of 130 kDa. Temperature and pH optima of this enzyme were 45 degrees C and 4.5, respectively. Substrate specificity tests revealed that the enzyme exerts only beta-D-mannosidase activity. The K(M) and V(max) values for p-nitrophenyl beta-D-mannopyranoside were determined to be 2.4 mM and 50.3 micromol min(-1)mg(-1), respectively. The catalytic efficiency of this beta-mannosidase (11,519 min(-1)) was significantly higher than those reported for beta-mannosidases from other sources. It was verified that this is an exo-acting glycosyl hydrolase with transglycosidase activity. When the enzyme was incubated in the presence of p-nitrophenyl beta-D-mannopyranoside, self-transfer of the mannosyl group was observed, and a 10-15% yield of a beta-1-4 disaccharide was obtained. When the reaction was performed in the presence of o-nitrophenyl alpha-D-2-deoxy-N-acetyl glucopyranoside in 3:1 molar ratio with respect to the p-nitrophenyl beta-D-mannopyranoside, two regioisomers (85:15, 12% yield) due to the beta-mannosylation of the heteroacceptor in 4 and in 6 positions were formed.

Publication types

  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Acetylglucosamine / analogs & derivatives
  • Acetylglucosamine / metabolism
  • Animals
  • Aplysia / enzymology*
  • Carbohydrate Conformation
  • Catalysis
  • Enzyme Stability
  • Hydrogen-Ion Concentration
  • Hydrolysis
  • Mannosides / metabolism
  • Substrate Specificity
  • Temperature
  • beta-Mannosidase / chemistry
  • beta-Mannosidase / isolation & purification*
  • beta-Mannosidase / metabolism*

Substances

  • Mannosides
  • 4-nitrophenyl-N-acetyl-2-deoxyglucopyranoside
  • 4-nitrophenyl-beta-D-mannopyranoside
  • beta-Mannosidase
  • Acetylglucosamine