Template-directed olefin cross metathesis

Org Lett. 2005 Sep 15;7(19):4213-6. doi: 10.1021/ol051599g.

Abstract

[reaction: see text] A template containing two secondary dialkylammonium ion recognition sites for encirclement by olefin-bearing dibenzo[24]crown-8 derivatives has been used to promote olefin cross metatheses with ruthenium-alkylidene catalysts. For monoolefin monomers, the rates of metatheses and yields of the dimers are both amplified in the presence of the template. Likewise, for a diolefin monomer, the yield of the dimer is enhanced in the presence of the template under conditions where higher oligomers are not formed.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't
  • Research Support, U.S. Gov't, Non-P.H.S.

MeSH terms

  • Alkenes / chemistry*
  • Catalysis
  • Chromatography, High Pressure Liquid
  • Dimerization
  • Molecular Structure
  • Ruthenium / chemistry

Substances

  • Alkenes
  • Ruthenium