Effects of DK-002, a synthesized (6aS,cis)-9,10-Dimethoxy-7,11b-dihydro-indeno[2,1-c]chromene-3,6a-diol, on platelet activity

Life Sci. 2006 Feb 2;78(10):1091-7. doi: 10.1016/j.lfs.2005.06.017. Epub 2005 Sep 8.

Abstract

In the present study, the mechanism of antiplatelet activity of DK-002, a synthesized (6aS,cis)-9,10-Dimethoxy-7,11b-dihydro-indeno[2,1-c]chromene-3,6a-diol, was investigated. DK-002 inhibited the thrombin, collagen, and ADP-induced rat platelet aggregation in a concentration-dependent manner, with IC50 values of 120, 27, and 47 microM, respectively. DK-002 also inhibited thrombin-induced dense granule secretion, thromboxane A2 synthesis, and [Ca2+]i elevation in platelets. DK-002 did not show any significant effect on ADP-induced inhibition of cyclic AMP elevation by prostaglandin E1, but DK-002 was confirmed to inhibit ADP-induced [Ca2+]i elevation and shape change. DK-002 inhibited 4-bromo-A23187-induced [Ca2+]i elevation in the presence of creatine phosphate/creatine phosphokinase (CP/CPK, a ADP scavenging system) and indomethacin (a specific inhibitor of cyclooxygenase). DK-002 also inhibited Ca2+ mobilization in thrombin- or 4-bromo-A23187-stimulated platelets through its inhibitory effects on both Ca2+ release from intracellular stores and Ca2+ influx, in the presence of CP/CPK and indomethacin. Taken together, the present study shows that DK-002 has inhibitory effects on stimulation of platelets, and suggests that its antiplatelet activity might be related to the inhibitory mechanism on Ca2+ mobilization in stimulated platelets.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adenosine Diphosphate / pharmacology
  • Animals
  • Benzopyrans / chemistry
  • Benzopyrans / pharmacology*
  • Blood Platelets / drug effects*
  • Blood Platelets / ultrastructure
  • Calcium / blood
  • Creatine Kinase / metabolism
  • Cyclic AMP / metabolism
  • Cyclooxygenase Inhibitors / pharmacology
  • Cytoplasmic Granules / drug effects
  • In Vitro Techniques
  • Indenes / chemistry
  • Indenes / pharmacology*
  • Indomethacin / pharmacology
  • Ionophores / pharmacology
  • Platelet Aggregation / drug effects*
  • Platelet Aggregation Inhibitors / pharmacology*
  • Rats
  • Rats, Sprague-Dawley
  • Serotonin / blood
  • Thrombin / pharmacology
  • Thromboxane B2 / blood

Substances

  • Benzopyrans
  • Cyclooxygenase Inhibitors
  • DK-002
  • Indenes
  • Ionophores
  • Platelet Aggregation Inhibitors
  • Serotonin
  • Thromboxane B2
  • Adenosine Diphosphate
  • Cyclic AMP
  • Creatine Kinase
  • Thrombin
  • Calcium
  • Indomethacin