Respiratory syncytial virus fusion inhibitors. Part 3: Water-soluble benzimidazol-2-one derivatives with antiviral activity in vivo

Bioorg Med Chem Lett. 2006 Mar 1;16(5):1115-22. doi: 10.1016/j.bmcl.2005.11.109. Epub 2005 Dec 20.

Abstract

The introduction of acidic and basic functionality into the side chains of respiratory syncytial virus (RSV) fusion inhibitors was examined in an effort to identify compounds suitable for evaluation in vivo in the cotton rat model of RSV infection following administration as a small particle aerosol. The acidic compounds 2r, 2u, 2v, 2w, 2z, and 2aj demonstrated potent antiviral activity in cell culture and exhibited efficacy in the cotton rat comparable to ribavirin. In a BALB/c mouse model, the oxadiazolone 2aj reduced virus titers following subcutaneous dosing, whilst the ester 2az and amide 2aab exhibited efficacy following oral administration. These results established the potential of this class of RSV fusion inhibitors to interfere with infection in vivo following topical or systemic administration.

MeSH terms

  • Amines / chemistry
  • Animals
  • Antiviral Agents / adverse effects
  • Antiviral Agents / chemical synthesis
  • Antiviral Agents / chemistry*
  • Antiviral Agents / pharmacology*
  • Benzimidazoles / adverse effects
  • Benzimidazoles / chemical synthesis
  • Benzimidazoles / chemistry*
  • Benzimidazoles / pharmacology*
  • Membrane Fusion / drug effects*
  • Mice
  • Molecular Structure
  • Rats
  • Respiratory Syncytial Viruses / drug effects*
  • Respiratory Syncytial Viruses / physiology*
  • Sigmodontinae
  • Solubility
  • Structure-Activity Relationship
  • Water / chemistry*

Substances

  • Amines
  • Antiviral Agents
  • Benzimidazoles
  • Water
  • benzimidazol-2-one