Morphology and surface plasma changes of Au-Pt bimetallic nanoparticles

J Nanosci Nanotechnol. 2006 May;6(5):1411-5. doi: 10.1166/jnn.2006.199.

Abstract

In this study, we examined the amount-dependent change in morphology in a series of Au-Pt bimetallic nanoparticles synthesized using chemical reduction. The amount of Au precursor was kept constant throughout the experiment. The Au/Pt molar ratio was varied from 1/1 to 1/4 to synthesize Pt shell layers with different thicknesses. We observed a remarkable shift of the surface plasmon band at around 410 nm. By high-resolution transmission electron microscopy (HRTEM) and energy-dispersive spectrometry (EDS), the composition of the shell layer was found to be Pt-enriched Au-Pt alloy. As the concentration of Pt increases, Pt clusters (ca. 1.8 nm in diameter) form a string-like shape on the surface of nanoparticles.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Alloys / chemistry*
  • Crystallization / methods*
  • Electrochemistry / methods
  • Gases / chemistry
  • Gold / chemistry*
  • Hot Temperature
  • Materials Testing
  • Metals / chemistry
  • Molecular Conformation
  • Nanostructures / chemistry*
  • Nanostructures / ultrastructure*
  • Nanotechnology / methods*
  • Particle Size
  • Platinum / chemistry*
  • Surface Properties

Substances

  • Alloys
  • Gases
  • Metals
  • Platinum
  • Gold