The effect of alpha-tocopherol on the oxidation and free radical decay in irradiated UHMWPE

Biomaterials. 2006 Nov;27(32):5580-7. doi: 10.1016/j.biomaterials.2006.07.017. Epub 2006 Aug 2.

Abstract

We developed a radiation cross-linked ultra-high molecular weight polyethylene (UHMWPE) stabilized with alpha-tocopherol (Vitamin E) as a bearing material in total joint replacements. The stabilizing effect of alpha-tocopherol on free radical reactions in UHMWPE is not well understood. We investigated the effect of alpha-tocopherol on the oxidation and transformation of residual free radicals during real-time aging of alpha-tocopherol-doped, irradiated UHMWPE (alphaTPE) and irradiated UHMWPE (control). Samples were aged at 22 degrees C (room temperature) in air, at 40 degrees C in air and at 40 degrees C in water for 7 months. During the first month, alphaTPE showed some oxidation at the surface, which stayed constant thereafter. Control exhibited substantial oxidation in the subsurface region, which increased with time. The alkyl/allyl free radicals transformed to oxygen centered ones in both materials; this transformation occurred faster in alpha-TPE. In summary, the real-time oxidation behavior of alpha-TPE was consistent with that observed using accelerated aging methods. This new UHMWPE is oxidation resistant and is expected to maintain its properties in the long term.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Electron Spin Resonance Spectroscopy
  • Free Radicals / chemistry
  • Hydrogen Peroxide / chemistry
  • Molecular Structure
  • Oxidation-Reduction / drug effects
  • Oxidation-Reduction / radiation effects
  • Polyethylenes / chemistry*
  • Polyethylenes / radiation effects*
  • Temperature
  • alpha-Tocopherol / chemistry*
  • alpha-Tocopherol / pharmacology*

Substances

  • Free Radicals
  • Polyethylenes
  • ultra-high molecular weight polyethylene
  • Hydrogen Peroxide
  • alpha-Tocopherol