Photoinduced charge transfer and efficient solar energy conversion in a blend of a red polyfluorene copolymer with CdSe nanoparticles

Nano Lett. 2006 Aug;6(8):1789-93. doi: 10.1021/nl061085q.

Abstract

We present measurements of charge transfer and the photovoltaic effect in a blend of the alternating polyfluorene copolymer poly(2,7-(9,9-dioctyl-fluorene)-alt-5,5-(4',7'-di-2-thienyl-2',1',3'-benzothiadiazole)) with branched CdSe nanoparticles. Quasi-steady-state photoinduced absorption measurements identified a long-lived charged species that formed after photoexcitation at room temperature. Photovoltaic devices based on this blend system showed a spectral response extending to 650 nm and gave a solar power conversion efficiency of 2.4% under Air Mass 1.5 Global (AM1.5G) conditions.

Publication types

  • Evaluation Study
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Cadmium Compounds / chemistry*
  • Cadmium Compounds / radiation effects
  • Electric Power Supplies*
  • Electrochemistry / instrumentation*
  • Electrochemistry / methods
  • Electron Transport
  • Energy Transfer
  • Equipment Design
  • Equipment Failure Analysis
  • Fluorenes / chemistry*
  • Fluorenes / radiation effects
  • Light
  • Nanostructures / chemistry*
  • Nanostructures / radiation effects
  • Nanotechnology / instrumentation
  • Nanotechnology / methods
  • Photochemistry / instrumentation*
  • Photochemistry / methods
  • Selenium Compounds / chemistry*
  • Selenium Compounds / radiation effects
  • Solar Energy*
  • Static Electricity
  • Transducers

Substances

  • Cadmium Compounds
  • Fluorenes
  • Selenium Compounds
  • fluorene
  • cadmium selenide