Optimization of the cellular import of functionally active SH2-domain-interacting phosphopeptides

Cell Mol Life Sci. 2006 Nov;63(22):2682-93. doi: 10.1007/s00018-006-6346-6.

Abstract

Phosphopeptides interacting with src homology 2 (SH2) domains can activate essential signaling enzymes in vitro. When delivered to cells, they may disrupt protein-protein interactions, thereby influencing intracellular signaling. We showed earlier that phosphopeptides corresponding to the inhibitory motif of Fcgamma receptor IIb and a motif of the Grb2-associated binder 1 adaptor protein activate SH2-containing tyrosine phosphatase 2 in vitro. To study the ex vivo effects of these peptides, we have now compared different methods for peptide delivery: (i) permeabilization of the target cells and (ii) the use of cell-permeable vectors, which are potentially able to transport biologically active compounds into B cells. We found octanoyl-Arg(8) to be an optimal carrier for the delivery of phosphopeptides to the cells. With this strategy, the function of cell-permeable SHP-2-binding phosphopeptides was analyzed. These peptides modulated the protein phosphorylation in B cells in a dose- and time-dependent manner.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Adaptor Proteins, Signal Transducing / metabolism
  • Amino Acid Motifs
  • B-Lymphocytes / metabolism*
  • Burkitt Lymphoma / metabolism*
  • Humans
  • Permeability
  • Phosphopeptides / chemistry
  • Phosphopeptides / metabolism*
  • Phosphopeptides / pharmacology*
  • Phosphoproteins / metabolism*
  • Phosphorylation
  • Phosphotyrosine / metabolism
  • Signal Transduction
  • src Homology Domains*

Substances

  • Adaptor Proteins, Signal Transducing
  • GAB1 protein, human
  • Phosphopeptides
  • Phosphoproteins
  • Phosphotyrosine