Thermal degradation of PCDD/F, PCB and HCB in municipal solid waste ash

Chemosphere. 2007 Mar;67(3):474-81. doi: 10.1016/j.chemosphere.2006.09.057. Epub 2006 Nov 15.

Abstract

A thermal degradation procedure for reducing the concentrations of mono- to octa-chlorinated PCDD/Fs, PCBs and hexa-chlorobenzenes (HCB) in filter ash from incinerated municipal solid waste (MSW) is described. Thermal treatment of filter ash samples at 500 degrees C for 60 min in a closed system providing low oxygen conditions resulted in 97% and 99% reductions in the total and I-TEQ concentrations of PCDD/Fs, to 6.8 microg kg(-1) ash and <0.05 microg I-TEQ kg(-1) ash, respectively. Increasing the thermal treatment time to 480 min, at the same temperature, yielded 99% reductions in both total and I-TEQ concentrations of the mono- to octa-chlorinated PCDD/Fs. Similar effects were observed for HCB and PCBs. The data from this study indicate that PCDD/Fs and other toxic organic compounds in ash from incinerated MSW, can be effectively degraded by this procedure, which combines relatively low-temperatures, short treatment times, and low oxygen conditions.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Benzofurans / chemistry*
  • Carbon / chemistry
  • Coal Ash
  • Dibenzofurans, Polychlorinated
  • Hexachlorobenzene / chemistry*
  • Hot Temperature*
  • Incineration / methods*
  • Particulate Matter / chemistry
  • Polychlorinated Biphenyls / chemistry*
  • Polychlorinated Dibenzodioxins / analogs & derivatives*
  • Polychlorinated Dibenzodioxins / chemistry

Substances

  • Benzofurans
  • Coal Ash
  • Dibenzofurans, Polychlorinated
  • Particulate Matter
  • Polychlorinated Dibenzodioxins
  • Hexachlorobenzene
  • Carbon
  • Polychlorinated Biphenyls