Disposition and metabolic profiling of bisphenol F in pregnant and nonpregnant rats

J Agric Food Chem. 2006 Dec 27;54(26):10307-14. doi: 10.1021/jf062250q.

Abstract

The distribution of bisphenol F (4,4'-dihydroxydiphenyl-methane, BPF) was studied in female Sprague-Dawley rats. Pregnant and nonpregnant animals were gavaged with a single dose of 7 or 100 mg/kg [3H]BPF and were kept for 96 h in metabolic cages. The excretion of BPF residues occurred mainly in urine (43-54% of the administered dose), which was found to contain at least six different metabolites, and to a lesser extent in feces (15-20% of the administered dose). Sulfatase treatment and subsequent high-performance liquid chromatography analyses suggest that the major urinary metabolite (more than 50% of the radioactivity present in urine) is a sulfate conjugate of BPF. At 96 h, BPF residues were detectable in all tissues examined with the largest amounts in the liver (0.5% of the dose). In pregnant rats dosed at day 17 of gestation, BPF residues were detected in the uterus, placenta, amniotic fluid, and fetuses (0.9-1.3% of the administered dose). Large amounts of radioactivity (8-10% of the dose) were still located in the digestive tract lumen at the end of the study. After administration of a single oral dose of [3H]BPF, 46% of the distributed radioactivity was excreted in bile over a 6 h period. In rats, BPF and/or its metabolites very likely undergo enterohepatic cycling, which could be responsible for the relatively high amounts of residues still excreted 4 days after BPF administration. This bisphenol is efficiently absorbed and distributed to the reproductive tract in female rats, and its residues pass the placental barrier at a late stage of gestation in rats.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Animals
  • Benzhydryl Compounds / administration & dosage
  • Benzhydryl Compounds / pharmacokinetics*
  • Benzhydryl Compounds / urine
  • Bile / metabolism
  • Chromatography, High Pressure Liquid
  • Drug Residues / analysis*
  • Female
  • Fetus / metabolism
  • Food Contamination
  • Placenta / chemistry
  • Pregnancy
  • Rats
  • Rats, Sprague-Dawley
  • Tritium
  • Uterus / chemistry

Substances

  • Benzhydryl Compounds
  • Tritium
  • 4,4'-bisphenol F