Sequential synthesis of type II colloidal CdTe/CdSe core-shell nanocrystals

Small. 2005 Mar;1(3):332-8. doi: 10.1002/smll.200400069.

Abstract

Colloidal type II CdTe/CdSe nanocrystals were synthesized by sequential addition of a tri-n-octylphosphine telluride (TOPTe)/TOP solution and several shell-precursor solutions to a CdO/TOP solution; the shell-precursor solutions consisted of CdO and TOPSe in TOP. For the growth of the CdTe core, the TOPTe/TOP solution was swiftly added to the CdO/TOP solution at a higher temperature (300 degrees C) than the growth temperature (250 degrees C). For the growth of the CdSe shell, in contrast, the CdO/TOPSe/TOP solution was slowly added to the CdTe/TOP solution at a lower temperature than the growth temperature (200-240 degrees C). The temporal evolution of the optical properties of the growing core-shell nanocrystals was monitored in detail. During the growth of the CdSe shell, the core-shell nanocrystals exhibited interesting changes in photoluminescence (PL) properties. The highest PL efficiency (approximately 38 %) was detected from core-shell nanocrystals with a CdSe shell thickness of 0.4-0.5 nm (indicated by TEM); the formation of the first monolayer is proposed. Our synthetic approach is well suited to a practical realization of engineering materials with bandgaps in the near-IR and IR spectral ranges.

MeSH terms

  • Cadmium Compounds / chemistry*
  • Colloids / chemistry*
  • Crystallization
  • Materials Testing
  • Metal Nanoparticles / chemistry*
  • Microscopy, Electron, Transmission
  • Nanoparticles
  • Selenium Compounds / chemistry*
  • Spectrophotometry
  • Spectrophotometry, Infrared
  • Tellurium / chemistry*
  • Temperature
  • Time Factors
  • X-Ray Diffraction

Substances

  • Cadmium Compounds
  • Colloids
  • Selenium Compounds
  • cadmium selenide
  • Tellurium
  • cadmium telluride