Instrumentation for medium-throughput two-dimensional capillary electrophoresis with laser-induced fluorescence detection

Anal Chem. 2007 Jan 15;79(2):765-8. doi: 10.1021/ac061652u.

Abstract

In two-dimensional capillary electrophoresis, a sample undergoes separation in the first dimension capillary by sieving electrophoresis. Fractions are periodically transferred across an interface into a second dimension capillary, where components are further resolved by micellar electrokinetic capillary electrophoresis. Previous instruments employed one pair of capillaries to analyze a single sample. We now report a multiplexed system that allows separation of five samples in parallel. Samples are injected into five first-dimension capillaries, fractions are transferred across an interface to 5 second-dimension capillaries, and analyte is detected by laser-induced fluorescence in a five-capillary sheath-flow cuvette. The instrument produces detection limits of 940 +/- 350 yoctomoles for 3-(2-furoyl)quinoline-2-carboxaldehyde labeled trypsin inhibitor in one-dimensional separation; detection limits degrade by a factor of 3.8 for two-dimensional separations. Two-dimensional capillary electrophoresis expression fingerprints were obtained from homogenates prepared from a lung cancer (A549) cell line, on the basis of capillary sieving electrophoresis (CSE) and micellar electrophoresis capillary chromatography (MECC). An average of 131 spots is resolved with signal-to-noise greater than 10. A Gaussian surface was fit to a set of 20 spots in each electropherogram. The mean spot width, expressed as standard deviation of the Gaussian function, was 2.3 +/- 0.7 transfers in the CSE dimension and 0.46 +/- 0.25 s in the MECC dimension. The standard deviation in spot position was 1.8 +/- 1.2 transfers in the CSE dimension and 0.88 +/- 0.55 s in the MECC dimension. Spot capacity was 300.

Publication types

  • Research Support, N.I.H., Extramural
  • Research Support, Non-U.S. Gov't

MeSH terms

  • Biogenic Amines / analysis*
  • Cell Line, Tumor
  • Chromatography, Micellar Electrokinetic Capillary
  • Electrophoresis, Capillary / instrumentation*
  • Fluorescence
  • Furans / analysis
  • Humans
  • Lasers
  • Lung Neoplasms
  • Proteins / analysis*
  • Quinolines / analysis
  • Sensitivity and Specificity
  • Spectrometry, Fluorescence / instrumentation*
  • Trypsin Inhibitors / analysis

Substances

  • Biogenic Amines
  • Furans
  • Proteins
  • Quinolines
  • Trypsin Inhibitors
  • 3-(2-furoyl)quinoline-2-carbaldehyde