An essential oligomannosidic glycan chain in the catalytic domain of autotaxin, a secreted lysophospholipase-D

J Biol Chem. 2007 Apr 13;282(15):11084-91. doi: 10.1074/jbc.M611503200. Epub 2007 Feb 16.

Abstract

Autotaxin/NPP2, a secreted lysophospholipase-D, promotes cell proliferation, survival, and motility by generating the signaling molecule lysophosphatidic acid. Here we show that ectonucleotide pyrophosphatase/phosphodiesterase 2 (NPP2) is N-glycosylated on Asn-53, Asn-410, and Asn-524. Mutagenesis and deglycosylation experiments revealed that only the glycosylation of Asn-524 is essential for the expression of the catalytic and motility-stimulating activities of NPP2. The N-glycan on Asn-524 was identified as Man8/9GlcNAc2, which is rarely present on mature eukaryotic glycoproteins. Additional studies show that this Asn-524-linked glycan is not accessible to alpha-1,2-mannosidase, suggesting that its non-reducing termini are buried inside the folded protein. Consistent with a structural role for the Asn-524-linked glycan, only the mutation of Asn-524 augmented the sensitivity of NPP2 to proteolysis and increased its mobility during Blue Native PAGE. Asn-524 is phylogenetically conserved and maps to the catalytic domain of NPP2, but a structural model of this domain suggests that Asn-524 is remote from the catalytic site. Our study defines an essential role for the Asn-524-linked glycan chain of NPP2.

Publication types

  • Research Support, Non-U.S. Gov't

MeSH terms

  • Amino Acid Sequence
  • Animals
  • Asparagine / genetics
  • Asparagine / metabolism
  • Carbohydrate Conformation
  • Catalytic Domain
  • Cell Line
  • Conserved Sequence
  • Enzyme Activation
  • Glycoside Hydrolases / metabolism
  • Glycosylation
  • Humans
  • Models, Molecular
  • Molecular Sequence Data
  • Mutation / genetics
  • Oligosaccharides / chemistry*
  • Oligosaccharides / metabolism*
  • Phosphoric Diester Hydrolases / chemistry*
  • Phosphoric Diester Hydrolases / genetics
  • Phosphoric Diester Hydrolases / metabolism*
  • Pyrophosphatases / chemistry*
  • Pyrophosphatases / genetics
  • Pyrophosphatases / metabolism*
  • Rats
  • Sequence Alignment

Substances

  • Oligosaccharides
  • oligomannoside
  • Asparagine
  • Phosphoric Diester Hydrolases
  • alkylglycerophosphoethanolamine phosphodiesterase
  • Glycoside Hydrolases
  • Pyrophosphatases