Identification of a small-molecule inhibitor of class Ia PI3Ks with cell-based screening

Chem Biol. 2007 Apr;14(4):371-7. doi: 10.1016/j.chembiol.2007.02.004.

Abstract

The mammalian target of rapamycin (mTOR) signaling network is central to the regulation of cell growth in response to both growth factors and nutrients. We developed a high-throughput, cell-based assay to identify small-molecule modulators of the mTOR signaling network. One such compound, which we name quinostatin, potently inhibits this network by directly targeting the lipid-kinase activity of the catalytic subunits of class Ia PI3Ks. This study illustrates the power of unbiased, phenotypic screening as a means for illuminating cell circuitry, and resulted in the identification of a chemotype for selective inhibition of the class Ia PI3Ks.

Publication types

  • Research Support, N.I.H., Extramural

MeSH terms

  • Catalytic Domain
  • Cell Line, Tumor
  • Heterocyclic Compounds, 3-Ring / chemistry
  • Heterocyclic Compounds, 3-Ring / isolation & purification*
  • Heterocyclic Compounds, 3-Ring / pharmacology*
  • Humans
  • Phosphatidylinositol 3-Kinases / chemistry
  • Phosphatidylinositol 3-Kinases / metabolism
  • Phosphoinositide-3 Kinase Inhibitors*
  • Phosphorylation / drug effects
  • Protein Kinases / metabolism
  • Quinolines / chemistry
  • Quinolines / isolation & purification*
  • Quinolines / pharmacology*
  • Ribosomal Protein S6 / metabolism
  • Ribosomal Protein S6 Kinases, 70-kDa / metabolism
  • Signal Transduction
  • Structure-Activity Relationship
  • TOR Serine-Threonine Kinases

Substances

  • Heterocyclic Compounds, 3-Ring
  • Phosphoinositide-3 Kinase Inhibitors
  • Quinolines
  • Ribosomal Protein S6
  • quinostatin
  • Protein Kinases
  • MTOR protein, human
  • Ribosomal Protein S6 Kinases, 70-kDa
  • TOR Serine-Threonine Kinases